Compressed glassy carbon: An ultrastrong and elastic interpenetrating graphene network

نویسندگان

  • Meng Hu
  • Julong He
  • Zhisheng Zhao
  • Timothy A Strobel
  • Wentao Hu
  • Dongli Yu
  • Hao Sun
  • Lingyu Liu
  • Zihe Li
  • Mengdong Ma
  • Yoshio Kono
  • Jinfu Shu
  • Ho-Kwang Mao
  • Yingwei Fei
  • Guoyin Shen
  • Yanbin Wang
  • Stephen J Juhl
  • Jian Yu Huang
  • Zhongyuan Liu
  • Bo Xu
  • Yongjun Tian
چکیده

Carbon's unique ability to have both sp2 and sp3 bonding states gives rise to a range of physical attributes, including excellent mechanical and electrical properties. We show that a series of lightweight, ultrastrong, hard, elastic, and conductive carbons are recovered after compressing sp2-hybridized glassy carbon at various temperatures. Compression induces the local buckling of graphene sheets through sp3 nodes to form interpenetrating graphene networks with long-range disorder and short-range order on the nanometer scale. The compressed glassy carbons have extraordinary specific compressive strengths-more than two times that of commonly used ceramics-and simultaneously exhibit robust elastic recovery in response to local deformations. This type of carbon is an optimal ultralight, ultrastrong material for a wide range of multifunctional applications, and the synthesis methodology demonstrates potential to access entirely new metastable materials with exceptional properties.

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عنوان ژورنال:

دوره 3  شماره 

صفحات  -

تاریخ انتشار 2017